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Polydimethylsiloxane (PDMS), also known as dimethylpolysiloxane or dimethicone, is a silicone polymer with a wide variety of uses, from cosmetics to industrial lubrication and passive daytime radiative cooling. [1] [2] [3] PDMS is particularly known for its unusual rheological (or flow) properties.
The formula to calculate average shear stress τ or force per unit area is: [1] =, where F is the force applied and A is the cross-sectional area.. The area involved corresponds to the material face parallel to the applied force vector, i.e., with surface normal vector perpendicular to the force.
Polydimethylsiloxane is a prevalent siloxane. In organosilicon chemistry, a siloxane is an organic compound containing a functional group of two silicon atoms bound to an oxygen atom: Si−O−Si. The parent siloxanes include the oligomeric and polymeric hydrides with the formulae H[OSiH 2] n OH and [OSiH 2] n. [1]
Elastic properties describe the reversible deformation (elastic response) of a material to an applied stress.They are a subset of the material properties that provide a quantitative description of the characteristics of a material, like its strength.
In the first developments of synthetic setae, polymers like polyimide, polypropylene and polydimethylsiloxane (PDMS) are frequently used since they are flexible and easily fabricated. Later, as nanotechnology rapidly developed, Carbon Nanotubes (CNTs) are preferred by most research groups and used in most recent projects.
Although the shear modulus, μ, must be positive, the Lamé's first parameter, λ, can be negative, in principle; however, for most materials it is also positive. The parameters are named after Gabriel Lamé. They have the same dimension as stress and are usually given in SI unit of stress [Pa].
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Nonlinear viscoelasticity also elucidates observed phenomena such as normal stresses, shear thinning, and extensional thickening in viscoelastic fluids. [ 3 ] An anelastic material is a special case of a viscoelastic material: an anelastic material will fully recover to its original state on the removal of load.